nice , maybe try to find out what he was playing through
beautiful tone indeed and very tasty playing too!
Following because im Interested
I would check out Tone Junkie profiles. They have that chimey, clean-but-not-clean thing going on in spades.
Also, I'd try adding Clean Boost in front of a breaking-up amp profile, to boost the gain with clarity, rather than Green Scream into a clean amp, which will just lose clarity. Or use Green Scream into a breaking up amp, with the gain off and the output volume right up.
Amp-wise, I'd try one of the Bogner Shiva profiles; it's a wonderful amp which really seems to lend itself to profiling well, and has a great, chimy-clean breakup sound.
Plus, of course, you need a good single coil neck pickup! That's a Strat p/u. Most Tele neck pickups probably won't get that sound.
I use my HPD profiles for these kinds of sounds. Works great.
Cheers,
Mats N
load the Tonejunkies FreePack and check the med gain crunch Rigs
you will find many suitings
my fav is the T Wreck Liverbird
I don’t know what guitar you are using but single coil neck pick up on a tele is key here.
Several of you beat me to it, but the first thing I heard was that it was played on a single coil neck pickup. Fantastic playing and tones. And the best looking non-Fender tele headstock I've seen, IMHO.
Bilinguitar, experiment with the compressor in the Amp section. That is probably your best way to get the sustain/feel that you are looking for.
I get a lot of mileage out of taking profiles that have more gain/are more distorted than I want, and turning the gain down. There is something that I really like about both the sound and the feel of those profiles with the gain reduced. Even with the gain all the way down, they are still fat. I've always guessed that this was a byproduct of how the profiling process works.
If you need to resort to driving the front end, try the pure boost.
Now, I'm going to go try Mats' HPD profiles and Tone Junkie's T Wreck Liverbird per digbob. 
